Publication Type
Journal
Journal Name
Physical Review Letters
Publication Date
Page Number
247202
Volume
125
Issue
24
Abstract
Bond-dependent magnetic interactions can generate exotic phases such as Kitaev spin-liquid states. Experimentally determining the values of bond-dependent interactions is a challenging but crucial problem. Here, I show that each symmetry-allowed nearest-neighbor interaction on triangular and honeycomb lattices has a distinct signature in paramagnetic neutron-diffraction data, and that such data contain sufficient information to determine the spin Hamiltonian unambiguously via unconstrained fits. Moreover, I show that bond-dependent interactions can often be extracted from powder-averaged data. These results facilitate experimental determination of spin Hamiltonians for materials that do not show conventional magnetic ordering.
