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Destabilization of Magnetic Order in a Dilute Kitaev Spin Liquid Candidate

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Publication Type
Journal
Journal Name
APS Physics
Publication Date
Conference Date
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The insulating honeycomb magnet αRuCl3 exhibits fractionalized excitations that signal its proximity to a Kitaev quantum spin liquid state; however, at T=0 , fragile long-range magnetic order arises from non-Kitaev terms in the Hamiltonian. Spin vacancies in the form of Ir3+ substituted for Ru are found to destabilize this long-range order. Neutron diffraction and bulk characterization of Ru1xIrxCl3 show that the magnetic ordering temperature is suppressed with increasing x , and evidence of zigzag magnetic order is absent for x>0.3 . Inelastic neutron scattering demonstrates that the signature of fractionalized excitations is maintained over the full range of x investigated. The depleted lattice without magnetic order thus hosts a spin-liquid-like ground state that may indicate the relevance of Kitaev physics in the magnetically dilute limit of RuCl3 .