April 2014

Journal

Molecular-Flow Properties of RIB Type Vapor-Transport Systems Using a Fast-Valve

By:
Alton, Gerald D; Bilheux, Hassina ; Zhang, Y.; Liu, Yuan
Journal Name:
Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms
Page Number:
30-39
Volume:
329
Issue Number:
n/a
Publication Date:
April 2014
View DOI Listing:
https://doi.org/10.1016/j.nimb.2014.02.129

Abstract

The advent of the fast-valve device, described previously, permits measurement of molecular-flow times of chemically active or inactive gaseous species through radioactive ion beam (RIB) target–ion–source systems, independent of size, geometry and materials of construction. Thus, decay losses of short-half-life RIBs can be determined for a given target/vapor-transport system in advance of on-line operation, thereby ascertaining the feasibility of the system design for successful processing of a given isotope. In this article, molecular-flow-time theory and experimentally measured molecular-flow time data are given for serial- and parallel-coupled Ta metal RIB vapor-transport systems similar to those used at ISOL based RIB facilities. In addition, the effect of source type on the molecular-flow time properties of a given system is addressed, and a chemical passivation method for negating surface adsorption enthalpies for chemically active gaseous species on Ta surfaces is demonstrated.


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