Altermagnetic and Dipolar Splitting of Magnons in FeF2

Abstract

FeF2 is a prototypical rutile antiferromagnet recently proposed as an altermagnet, with a magnetic symmetry that permits spin-split electronic bands and chiral magnons. Using very-high-resolution inelastic neutron scattering on a single crystal of FeF2, we show that the dominant source of magnon splitting is in fact the long-range dipolar interaction rather than altermagnetic exchange terms. At momenta where the dipolar splitting vanishes, we observe additional broadening due to altermagnetic chiral splitting and estimate this splitting to be ∼35  μ⁢eV. Polarized measurements further reveal that, where dipolar splitting is present, the chiral magnon modes become mixed and the resulting modes are predominantly linearly polarized, with at most a small chiral component. These findings highlight the significant effect of dipolar interactions on magnon chirality, particularly when altermagnetic interactions are weak.