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Local magnetic cluster size identified by neutron total scattering in the site-diluted spin glass SnxFe4−xN (x=0.88)...

by Yuanpeng Zhang, Tanja Scholz, Richard Dronskowski, Marshall T Mcdonnell, Matthew G Tucker
Publication Type
Journal
Journal Name
Physical Review B
Publication Date
Page Number
014419
Volume
100
Issue
1

A detailed structure analysis for the site-diluted SnxFe4−xN (x=0.25, 0.41, and 0.88) has been carried out through complex modeling of the neutron total scattering data. We present quantitative evidence showing the local ferromagnetic cluster size extending to ∼8 Å on average when Sn0.88Fe3.12N undergoes the spin-glass transition (the other two not showing such a transition). The modeling methodology used in this work involving the corefinement of the nuclear and magnetic structure in both real and reciprocal space can potentially be applied generally to explore a variety of spin-glass material problems.