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Coherent Hopping Transport and Giant Negative Magnetoresistance in Epitaxial CsSnBr 3

Publication Type
Journal
Journal Name
ACS Applied Electronic Materials
Publication Date
Page Numbers
2948 to 2952
Volume
3
Issue
7

Single-crystal inorganic halide perovskites are attracting interest for quantum device applications. Here we present low-temperature quantum magnetotransport measurements on thin film devices of epitaxial single-crystal CsSnBr3, which exhibit two-dimensional Mott variable range hopping (VRH) and giant negative magnetoresistance. These findings are described by a model for quantum interference between different directed hopping paths, and we extract the temperature-dependent hopping length of charge carriers, their localization length, and a lower bound for their phase coherence length of ∼100 nm at low temperatures. These observations demonstrate that epitaxial halide perovskite devices are emerging as a material class for low-dimensional quantum coherent transport devices.