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Nuclear physicists at ORNL have identified a novel form of radioactivity predicted by theory—simultaneous emission of two protons from a decaying atomic nucleus.

New Type of Radioactivity Discovered at ORNL

Based on preliminary experiments at ORNL's Holifield Radioactive Ion Beam Facility (HRIBF), nuclear physicists have identified a new form of radioactivity—simultaneous emission of two protons from the decaying nucleus of an atom. The discovery of the protons, which may have been initially bound together in an ephemeral helium-2 nucleus as they were emitted from a neon-18 nucleus, is significant. It will allow physicists to better understand the strong nuclear force that holds protons and neutrons together in the nucleus, countering the repulsive Coulomb force that drives protons apart because of their like charges. Information about the energy levels and other properties of the emitted pair of protons will help scientists determine how protons are bound together in the nucleus and how they interact with each other and with neutrons.

"The nucleus is sending us a message about how it is put together," says Jim Beene, director of HRIBF, the only two-accelerator facility for producing radioactive ion beams in the United States.

"This is the first time that two-proton emission has been observed," says Witold Nazarewicz, deputy director of science at HRIBF, a leading theorist in nuclear structure physics, and a professor of nuclear physics at the University of Tennessee at Knoxville (UTK). "Experimenters at the Holifield facility have already discovered five radionuclides that emit single protons through decay." Nazarewicz makes calculations to describe the decay of one-proton emitters and is developing theory to describe two-proton emitters.

Led by George Gomez del Campo of ORNL's Physics Division, a group of ORNL and UTK physicists discovered two-proton emission from the decay of neon-18 nuclei formed in an experiment at HRIBF. Fluorine-17 ions in an intense, difficult-to-produce HRIBF beam bombarded hydrogen atoms (protons) in a polypropylene target. For the most part, protons were scattered from the bombarded target. Once in a billion encounters, a fluorine ion captured a proton in the target, forming neon-18.

One particular quantum state of neon-18, with an energy just over 6 million electron volts (MeV), was found to decay about one time out of 3000 by emitting two protons simultaneously to form oxygen-16. The remaining 2999 times it decayed by emitting a single proton to form fluorine-17.

Future experiments at the HRIBF (jpg, 33K)
Future experiments at the HRIBF could determine whether the neon-18 nucleus can decay by forming an oxygen-16 nucleus and helium-2 nucleus that breaks apart instantly into two protons, or whether the neon-18 undergoes a direct, three-body breakup into oxygen-16 and two protons, sometimes called democratic decay.

"We still have to answer a key question," Nazarewicz says. "Were the two protons leaving the neon-18 nucleus closely coupled together to form helium-2, or were they emitted almost independently in a direct three-body breakup into oxygen-16 and two protons, sometimes called 'democratic' decay? Even if the protons were emitted as a helium-2 nucleus, they would fly apart almost instantly. Our data favor the helium-2 emission, but a further experiment will be required to definitively distinguish between the two possibilities."

Two-proton (helium-2) decay was predicted in 1960 by the Russian theorist V. I. Goldanski. In the succeeding 40 years many efforts have been made to identify this elusive process definitively, but none have succeeded. These searches have invariably found sequential emission of single protons, through an intermediate state, instead of simultaneous two-proton emission (either as helium-2 or "democratically").

"For states of neon-18 up to 6.4 MeV," Nazarewicz says, "two protons can be emitted along with oxygen-16 only if they are emitted simultaneously. The sequential one-proton emission process is not possible, because no appropriate intermediate state exists."

The identification of two-proton emissions is important, but it will be especially significant if the emitted protons come out bound together and then separate, providing information on how they are entangled in their original state inside the neon-18 nucleus.

At HRIBF five single-proton emitters have been discovered by researchers led by ORNL's Krzysztof Rykaczewski. The proton-rich nuclides are holmium-140 (140Ho), holmium-141m (141mHo), thulium-145 (145Tm), lutetium-150m (150mLu), and lutetium-151m (151mLu).

"Of the single-proton emitters, we found that thulium-145 has the shortest half-life yet measured for proton radioactivity," Rykaczewski says. "It decays in 3.5 microseconds to form another radionuclide, erbium-144."

Nuclear physicists at HRIBF also discovered that thulium-146 breaks down into erbium-145 (145Er), releasing protons of different energies. In this case, Rykaczewski says, the observed proton fine structure offers a tool for studying neutron states in exotic nuclei.

Rykaczewski is looking forward this year to HRIBF's first radioactive ion beams for nuclear structure physics research—a proton-rich, nickel-56 beam, as well as neutron-rich beams. These beams will help nuclear physicists explore uncharted territory as these scientists create and discover some of the 3000 neutron-rich and proton-rich radioactive nuclides believed to exist when conditions are right. Recently commissioned digital signal processing electronics should help researchers reach this goal.

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